Supplement of Atmos. Chem. Phys., 14, 9137–9153, 2014 http://www.atmos-chem-phys.net/14/9137/2014/ doi:10.5194/acp-14-9137-2014-supplement © Author(s) 2014. CC Attribution 3.0 License. Supplement of Ozone vegetation damage effects on gross primary productivity in the United States X. Yue and N. Unger Correspondence to: X. Yue ([email protected]) Table S1. Match of model PFTs with that from NACP sites and the ISLSCP dataset. PFTs in the model PFTs at NACP sites PFTs from ISLSCP ID PFTs ID ID 1 Tundra 2 C3 grassland 3 C4 grassland 4 Shrubland PFTs N/A I PFTs N/A Grasslands a Grasslands N/A b Savannas II Closed Shrubland c Closed Shrubland III Woody Savannas d Open Shrubland IV Permanent Wetlands e Woody Savannas f Permanent Wetlands g Deciduous Broadleaf Forest 5 Deciduous Broadleaf Forest V Deciduous Broadleaf Forest h Deciduous Needleleaf Forest 6 Evergreen Needleleaf Forest VI Evergreen Needleleaf Forest i Evergreen Needleleaf Forest VII Mixed Forests j Mixed Forests N/A k Evergreen Broadleaf Forest Croplands (C4) l Croplands (C3/C4) m Cropland/Natural vegetation mosaic (C3/C4) 7 Tropical Rainforest 8 Cropland VIII NACP sites Fig. S1. Distribution of 40 North American Carbon Program (NACP) sites. The color indicates different land types as evergreen needleleaf forest (ENF, blue), deciduous broadleaf forest (DBF, magenta), grasslands (GRA, green), croplands (CRO, red), shrublands (SHR, yellow). “Mixed Forests” are classified as ENF, “Permanent Wetlands” and “Woody Savannas” as SHR (Table S1). The local vegetation type at each site is described in appendix Table A. Land Cover from ISLSCP Water Savannas Evergreen Needleleaf Forest Grasslands Evergreen Broadleaf Forest Permanent Wetlands Deciduous Needleleaf Forest Croplands Deciduous Broadleaf Forest Urban and Build-up Mixed Forests Cropland/Natural vegetation mosaic Closed Shrubland Snow and Ice Open Shrubland Barren or Sparsely vegetated Woody Savannas Unclassified Fig. S2. Land cover types in North America developed by the International Satellite Land-Surface Climatology Project (ISLSCP). CA−Ca1 (125.3oW, 49.9oN) CA−Ca2 (125.3oW, 49.9oN) CA−Ca3 (124.9oW, 49.5oN) 6 6 6 ENF 4 ENF 4 2 0 J A J o o 0 J A J J 0 J O o 6 ENF A J A J 0 J O CA−SJ2 (104.6oW, 53.9oN) CA−SJ3 (104.6oW, 53.9oN) 6 6 6 ENF ENF 4 2 0 J A J o US−Dk3 (79.1 W, 36 N) 6 0 J O o US−Ho1 (68.7 W, 45.2 N) ENF 4 2 J o 6 ENF 4 A 0 J A J 0 J O o o 4 2 0 J 0 J J O CA−Oas (106.2oW, 53.6oN) 6 A J A J o US−UMB (84.7 W, 45.6 N) 8 6 DBF 4 2 0 J A o A J O US−MMS (86.4oW, 39.3oN) o A A J 0 J O o CA−Mer (75.5 W, 45.4 N) o 0 J A J 0 J O o o A J 0 J O o US−Ton (121 W, 38.4 N) o 2 0 J A J 0 J O o o US−IB1 (88.2 W, 41.9 N) 4 2 0 J A J O J o o 4 2 0 J 0 J J O A J O GRA 2 A J 0 J O o US−Ne2 (96.5 W, 41.2 N) 2 A O US−Var (121oW, 38.4oN) 4 GRA o 6 CRO J GRA 0 J O US−Shd (96.7 W, 36.9 N) 0 J O US−Ne1 (96.5 W, 41.2 N) 4 J o 4 o 6 CRO A 2 A A 2 6 GRA 2 O CA−Let (112.9oW, 49.7oN) 4 SHR 0 J O US−IB2 (88.2 W, 41.8 N) 4 GRA 4 J o US−ARM (97.5 W, 36.6 N) 6 A J SHR 4 2 2 A 2 4 SHR O CA−WP1 (112.5oW, 55oN) 6 SHR o US−SO2 (116.6 W, 33.4 N) J DBF 4 o 0 J O O 2 4 o J US−MOz (92.2oW, 38.7oN) 6 DBF 6 J A US−Syv (89.3oW, 46.2oN) 8 6 ENF 4 2 0 J A 2 2 SHR 0 J O ENF 0 J O DBF 0 J o US−Los (90 W, 46.1 N) 4 J 2 O J US−PFa (90.3 W, 45.9 N) US−WCr (90.1 W, 45.8 N) 4 J A o 4 o 6 o 6 A ENF 2 2 0 J O o 4 ENF 6 DBF O 4 0 J O J US−Me3 (121.6oW, 44.3oN) 4 2 0 J o A US−Me2 (121.6 W, 44.5 N) 6 US−Ha1 (72.2oW, 42.5oN) 4 2 o O ENF 0 J O 2 6 DBF 4 J o 0 J O ENF 2 A J US−NR1 (105.5 W, 40 N) 4 ENF A o US−Me5 (121.6 W, 44.4 N) A 2 2 J 2 2 0 J O o A CA−TP4 (80.4oW, 42.7oN) 4 ENF 4 2 O ENF 4 CA−SJ1 (104.7oW, 53.9oN) 4 J 2 0 J O A CA−Qfo (74.3oW, 49.7oN) CA−Ojp (104.7 W, 53.9 N) 2 0 J O A o 4 ENF 2 2 2 0 J O CA−Obs (105.1 W, 54 N) 4 ENF 4 J o CA−NS1 (124.9 W, 49.5 N) 6 A ENF 4 2 0 J O o ENF 4 2 CA−Gro (82.2oW, 48.2oN) 6 6 CRO A J O US−Ne3 (96.4oW, 41.2oN) 4 CRO 2 A J O 0 J A J O Fig. S3. Comparison of monthly mean leaf area index (LAI, m2 m-2) from the Modern Era-Retrospective Analysis (MERRA) reanalysis (red solid lines) and the Moderate Resolution Imaging Spectroradiometer (MODIS) (blue dashed lines) at each NACP site. The name and location (longitude, latitude) are shown in the title. The land types include evergreen needleleaf forest (ENF), deciduous broadleaf forest (DBF), shrublands (SHR), grasslands (GRA), and croplands (CRO). o o CA−Ca1 (125.3 W, 49.9 N) 15 ENF 10 o o CA−Ca2 (125.3 W, 49.9 N) 10 ENF 0 J A J o o o ENF 0 J A J o CA−SJ1 (104.7 W, 53.9 N) 10 5 A J o CA−SJ2 (104.6 W, 53.9 N) A J 15 J 0 J A J o 10 5 J o A J o CA−Oas (106.2 W, 53.6 N) 15 J o 0 J A J o US−UMB (84.7 W, 45.6 N) 15 J A J 10 J A o 5 A J 0 J O o A J 0 J O o o A J 0 J O o CA−Mer (75.5 W, 45.4 N) 10 5 A J 0 J A J 0 J O o o US−IB1 (88.2 W, 41.9 N) 20 CRO 0 J o US−Ne1 (96.5 W, 41.2 N) J O 0 J J o J O O J O GRA 5 A J 0 J O o o US−Ne2 (96.5 W, 41.2 N) 0 J A US−Var (121oW, 38.4oN) 10 GRA CRO A J O US−Ne3 (96.4oW, 41.2oN) 20 CRO 10 10 A J GRA 0 J O US−Shd (96.7 W, 36.9 N) 20 10 A A o 30 CRO A 5 0 J O o 20 10 J O CA−Let (112.9oW, 49.7oN) 10 5 A J SHR 0 J O SHR 10 5 A 5 15 GRA O CA−WP1 (112.5oW, 55oN) 10 SHR US−Ton (121oW, 38.4oN) o J 5 0 J O A DBF 10 o US−IB2 (88.2 W, 41.8 N) 15 GRA J o US−ARM (97.5 W, 36.6 N) 10 A O US−MOz (92.2oW, 38.7oN) 15 5 0 J J ENF 10 DBF 10 SHR A 5 0 J O O US−Syv (89.3oW, 46.2oN) 15 ENF 10 J J ENF 0 J O 5 5 SHR A US−MMS (86.4 W, 39.3 N) US−SO2 (116.6oW, 33.4oN) A US−Me3 (121.6oW, 44.3oN) 10 o o DBF 0 J O US−Los (90oW, 46.1oN) 0 J O US−PFa (90.3 W, 45.9 N) 0 J O 5 0 J J o US−WCr (90.1 W, 45.8 N) 10 5 A o 15 DBF 10 A 5 0 J O o O 5 10 5 J ENF 10 ENF 15 DBF A CA−TP4 (80.4oW, 42.7oN) 15 US−Me2 (121.6oW, 44.5oN) 0 J O US−Ha1 (72.2 W, 42.5 N) 10 5 A o 5 10 o 15 DBF 10 o 5 0 J O o O ENF 0 J O ENF 15 ENF 5 0 J J CA−SJ3 (104.6 W, 53.9 N) 0 J O US−NR1 (105.5 W, 40 N) 10 ENF A o US−Me5 (121.6 W, 44.4 N) A 5 0 J O o J o 10 o 10 5 A CA−Qfo (74.3 W, 49.7 N) 5 0 J O ENF 10 5 A US−Ho1 (68.7oW, 45.2oN) 15 ENF 10 o 5 0 J O US−Dk3 (79.1oW, 36oN) 0 J O ENF 10 ENF 5 0 J J CA−Ojp (104.7 W, 53.9 N) 0 J O o 10 ENF A 5 0 J O o ENF 10 o 10 5 5 o 5 0 J O CA−Obs (105.1 W, 54 N) 10 ENF 10 J o CA−NS1 (124.9 W, 49.5 N) 15 A o CA−Gro (82.2 W, 48.2 N) 15 5 0 J O o ENF 10 5 5 o CA−Ca3 (124.9 W, 49.5 N) 15 A J O 0 J A J -2 O -1 Fig. S4. Comparison of long-term monthly mean GPP (g [C] m day ) from observations (blue points with error bars indicating one standard deviation) and the O3free simulations (black lines with shadings indicating one standard deviation) averaged over measurement period at each site. The simulation, METsite_LAImerra, is driven with meteorological forcings from MERRA and site measurements. The LAI is from MERRA. The name and location (longitude, latitude) are shown in the title. The land types include evergreen needleleaf forest (ENF), deciduous broadleaf forest (DBF), shrublands (SHR), grasslands (GRA), and croplands (CRO). Observed JJA GPP (g [C] m−2 d−1) 18 w/o ozone effect r = 0.81 15 high ozone effect r = 0.80 12 9 6 3 0 0 3 6 9 12 15 −2 −1 Simulated JJA GPP (g [C] m d ) 18 Fig. S5. Comparison of simulated summer average GPP without O3 damage (blue) and with O3 damage (red) with observations at 40 NACP sites. 0 −2 −2 US−Dk3 CA−Ca1 US−Ne1 US−Me2 US−Ha1 CA−Gro CA−TP4 US−Ho1 US−NR1 US−Me3 US−PFa US−Ton CA−Ca2 US−MOz US−UMB US−SO2 US−Ne2 US−IB1 CA−WP1 US−Syv CA−Ca3 US−MMS US−Ne3 US−IB2 US−WCr US−Me5 US−Shd CA−Obs CA−Qfo US−Los CA−Oas US−ARM CA−SJ3 CA−Ojp CA−Mer CA−Let CA−NS1 US−Var CA−SJ1 CA−SJ2 2 10 US−Dk3 CA−Ca1 US−Ne1 US−Me2 US−Ha1 CA−Gro CA−TP4 US−Ho1 US−NR1 US−Me3 US−PFa US−Ton CA−Ca2 US−MOz US−UMB US−SO2 US−Ne2 US−IB1 CA−WP1 US−Syv CA−Ca3 US−MMS US−Ne3 US−IB2 US−WCr US−Me5 US−Shd CA−Obs CA−Qfo US−Los CA−Oas US−ARM CA−SJ3 CA−Ojp CA−Mer CA−Let CA−NS1 US−Var CA−SJ1 CA−SJ2 2 15 US−Dk3 CA−Ca1 US−Ne1 US−Me2 US−Ha1 CA−Gro CA−TP4 US−Ho1 US−NR1 US−Me3 US−PFa US−Ton CA−Ca2 US−MOz US−UMB US−SO2 US−Ne2 US−IB1 CA−WP1 US−Syv CA−Ca3 US−MMS US−Ne3 US−IB2 US−WCr US−Me5 US−Shd CA−Obs CA−Qfo US−Los CA−Oas US−ARM CA−SJ3 CA−Ojp CA−Mer CA−Let CA−NS1 US−Var CA−SJ1 CA−SJ2 2 (a) (b) (c) 2 2 2 for each site ENF DBF SHR GRA CRO 5 2 for each site with low ozone effect 1 0 −1 2 for each site with high ozone effect 1 0 −1 Fig. S6. The calculated (a) χ2 of GPP and changes in χ2 after the inclusion of O3 damage impact with (b) low and (c) high O3 sensitivity at each site. The sites are sorted according to the values of χ2 in (a). The land cover definitions are: GRA, Grasslands; CRO, Croplands; ENF, Evergreen Needleleaf Forest; DBF, Deciduous Broadleaf Forest; SHR, Shrubland. See section 2.2.1 for the definition of χ2. (a) JJA mean Ozone from GCM (b) JJA mean Ozone from CASTNET o o 50 N 50 N 40oN 40oN 30oN 30oN 120oW 110oW 100oW 90oW 80oW 70oW 120oW 110oW 100oW 90oW 80oW 70oW (c) JJA MDA8 Ozone from GCM o 50 N 20 30 (d) JJA MDA8 Ozone from AIRDATA 40 50 o 50 N 40oN 40oN 30oN 30oN 120oW 110oW 100oW 90oW 80oW 20 30 70oW 40 60 70 80 (ppbv) 120oW 110oW 100oW 90oW 80oW 50 60 70 80 70oW (ppbv) Fig. S7. Comparison of summertime surface (a, b) diurnal mean and (c, d) daily maximum 8-hour average ozone between (a, c) GCM and observations from (b) CASTNET and (d) AIRDATA. (a) JJA GPP with high ozone damage (b) JJA GPP from NACP sites o o 50 N 50 N 40oN 40oN 30oN 30oN 120oW 110oW 100oW 90oW 2 80oW 4 70oW 6 120oW 110oW 100oW 90oW 8 10 12 14 80oW 70oW (g m-2 day-1) Fig. S8. Comparison of summertime GPP from (a) simulations with high ozone damage effects and (b) in situ measurements from NACP.
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