Copyright by the AIP Publishing. Asryan, Levon V.; Wu, Yuchang; Suris, Robert A., "Carrier capture delay and modulation bandwidth in an edge-emitting quantum dot laser," Appl. Phys. Lett. 98, 131108 (2011); http://dx.doi.org/10.1063/1.3571295 Carrier capture delay and modulation bandwidth in an edge-emitting quantum dot laser Levon V. Asryan, Yuchang Wu, and Robert A. Suris Citation: Applied Physics Letters 98, 131108 (2011); doi: 10.1063/1.3571295 View online: http://dx.doi.org/10.1063/1.3571295 View Table of Contents: http://scitation.aip.org/content/aip/journal/apl/98/13?ver=pdfcov Published by the AIP Publishing Articles you may be interested in Effect of excited states on the ground-state modulation bandwidth in quantum dot lasers Appl. Phys. Lett. 102, 191102 (2013); 10.1063/1.4804994 Influencing modulation properties of quantum-dot semiconductor lasers by carrier lifetime engineering Appl. Phys. Lett. 101, 131107 (2012); 10.1063/1.4754588 Effect of internal optical loss on the modulation bandwidth of a quantum dot laser Appl. Phys. Lett. 100, 131106 (2012); 10.1063/1.3697683 Upper limit for the modulation bandwidth of a quantum dot laser Appl. Phys. Lett. 96, 221112 (2010); 10.1063/1.3446968 Single-mode submonolayer quantum-dot vertical-cavity surface-emitting lasers with high modulation bandwidth Appl. Phys. Lett. 89, 141106 (2006); 10.1063/1.2358114 This article is copyrighted as indicated in the article. Reuse of AIP content is subject to the terms at: http://scitation.aip.org/termsconditions. Downloaded to IP: 128.173.125.76 On: Tue, 01 Apr 2014 19:24:05 APPLIED PHYSICS LETTERS 98, 131108 共2011兲 Carrier capture delay and modulation bandwidth in an edge-emitting quantum dot laser Levon V. Asryan,1,a兲 Yuchang Wu,1,b兲 and Robert A. Suris2,c兲 1 Virginia Polytechnic Institute and State University, Blacksburg, Virginia 24061, USA Ioffe Physico-Technical Institute, Saint Petersburg 194021, Russia 2 共Received 1 March 2011; accepted 8 March 2011; published online 30 March 2011兲 We show that the carrier capture from the optical confinement layer into quantum dots 共QDs兲 can strongly limit the modulation bandwidth −3 dB of a QD laser. As a function of the cross-section n of carrier capture into a QD, −3 dB asymptotically approaches its highest value when n → ⬁ 共the case of instantaneous capture兲. With reducing n, −3 dB decreases and becomes zero at a certain nonvanishing min n . The use of multiple-layers with QDs significantly improves the laser modulation response—−3 dB is considerably higher in a multilayer structure as compared to a single-layer structure at the same dc current. © 2011 American Institute of Physics. 关doi:10.1063/1.3571295兴 Due to the quantum-size effect, reducing dimensionality of the active region has been a key to developing lowthreshold semiconductor lasers.1,2 In commercial diode lasers, a two-dimensional 共2D兲 active region 关quantum well 共QW兲兴 is used.3,4 In quantum dot 共QD兲 lasers, an ultimate case of a zero-dimensional active region is realized.5,6 The interesting physics involved and the potential for wide range of applications have motivated extensive studies of QD lasers. However, in contrast to the steady-state characteristics, the dynamic properties of QD lasers need to be further scrutinized. In particular, the potential of QD lasers for highspeed direct modulation of the output optical power by injection current should be clarified. In Ref. 7, the highest modulation bandwidth attainable in QD lasers was estimated. For this purpose, an idealized situation of instantaneous carrier capture into QDs was assumed. In actual semiconductor lasers, carriers are not directly injected into the quantum-confined active region— they are first injected into the optical confinement layer 共OCL兲 and then captured into the active region 共Fig. 1兲. Indirect injection adversely affects the laser operating characteristics—the threshold current is increased8 and more temperature-sensitive,9 and the output optical power is decreased.10,11 Due to a transport delay across the OCL and a capture delay from the OCL into the active region, the bandwidth of direct modulation of the output power by injection current is also reduced 共see, e.g., Ref. 12 for QW lasers兲. In this letter, we briefly report on the effect of noninstantaneous capture of carriers into QDs on the modulation bandwidth of an edge-emitting QD laser. Our model is based on the following set of three coupled rate equations for free carriers in the OCL, carriers confined in QDs, and photons: 冉 冊 NS NS NS 2 f n = nvn 共1 − f n兲nOCL − nvnn1 f n t b b b − NS f 2n − vggmax共2f n − 1兲nph , b QD nph = vggmax共2f n − 1兲nph − vgnph , t 共2兲 共3兲 where nOCL is the free carrier density in the OCL, j is the injection current density, b is the OCL thickness, n is the cross-section of carrier capture into a QD, vn is the carrier thermal velocity, NS is the surface density of QDs, f n is the occupancy of the energy-level of a carrier confined in a QD, B is the spontaneous radiative recombination constant for the OCL, QD is the spontaneous radiative time in a QD, vg is the group velocity of light, gmax is the maximum modal gain,8 nph is the photon density 共per unit volume of the OCL兲 in the lasing mode,  = 共1 / L兲ln共1 / R兲 is the mirror loss, L is the cavity length, and R is the facet reflectivity. In Eqs. 共1兲 and 共2兲, the quantity n1 = N3D c exp共−En / T兲 characterizes the carrier thermal escape from a QD to the OCL, where N3D c is the effective density of states in the OCL, En is the carrier thermal excitation energy from a QD, and T is the temperature 共in units of energy兲. Strictly speaking, n is the only parameter adequately describing the capture/escape into/from a QD. Using n, two distinct characteristic times can be introduced—the capture time into an unoccupied QD ensemble11 and the thermal escape time from an individual QD,8,11 nOCL NS NS j = − nvn 共1 − f n兲nOCL + nvnn1 f n t eb b b 2 − BnOCL , 共1兲 a兲 Electronic mail: [email protected]. Electronic mail: [email protected]. c兲 Electronic mail: [email protected]. b兲 FIG. 1. Indirect injection into the active region of a QD laser. 0003-6951/2011/98共13兲/131108/3/$30.00 98,is131108-1 © 2011 American InstituteDownloaded of Physics to IP: This article is copyrighted as indicated in the article. Reuse of AIP content subject to the terms at: http://scitation.aip.org/termsconditions. 128.173.125.76 On: Tue, 01 Apr 2014 19:24:05 Appl. Phys. Lett. 98, 131108 共2011兲 Asryan, Wu, and Suris NS b 冊 −1 , esc = 共nvnn1兲−1 . 共4兲 In a specific structure considered below, capt,0 = 1.63 ps and esc = 0.07 ps at n = 10−11 cm2. We consider the spontaneous radiative recombination as the only mechanism of nonstimulated recombination in the OCL and QDs. The inclusion of the nonradiative Auger recombination will increase the threshold current density and the steady-state carrier density in the OCL, and, within the framework of the small-signal analysis, will decrease the differential nonstimulated recombination time, while not otherwise affecting the main derivations of this letter. Our model does not include the wetting layer 共WL兲, which is inherently present in self-assembled Stranski– Krastanow grown QD structures. The WL can affect the carrier capture into QDs. In addition to the direct capture from the bulk OCL into QDs, carriers will also be captured from the OCL into the 2D WL and then from the WL into QDs. The inclusion of the WL will thus require a careful consideration of all these capture processes. Due to inhomogeneous broadening of the transition energy in a QD-ensemble in an edge-emitting laser, we do not also consider the optical mode resonance with the QDtransition. This resonance in the context of QD nanocavity lasers was considered in Ref. 13. Applying the small-signal analysis of rate equations, we consider the injection current density in Eq. 共1兲 in the form of j = j0 + 共␦ jm兲exp共it兲, where j0 is the dc component and the amplitude ␦ jm of the time-harmonic ac component is small 共␦ jm Ⰶ j0 − jth, where jth is the threshold current density兲. We correspondingly look for nOCL, f n, and nph in Eqs. 共1兲–共3兲 in the form of nOCL = nOCL,0 + 共␦nOCL−m兲exp共it兲, f n = f n,0 + 共␦ f n−m兲exp共it兲, and nph = nph,0 + 共␦nph−m兲exp共it兲, where nOCL,0, f n,0, and nph,0 are the solutions of the steadystate rate equations at j = j0.10,11 In particular, f n,0 = 冉 冊 冉 冊 1 1 1  1 + max = 1 + , 2 2 g phvggmax 共5兲 where the photon lifetime in the cavity is ph = 1 L . = vg vg ln共1/R兲 共6兲 20 (GHz) 冉 capt,0 = nvn j0 = 63.8 kA/cm ω-3 dB / 2π 131108-2 10 2 2 10 kA/cm 2 1 kA/cm 0 0 5 10 σn (x10-11cm2) FIG. 2. Modulation bandwidth vs capture cross-section into a QD at different values of the dc component j0 of the injection current density in a single-layer structure. The horizontal dashed lines show −3 dB for the case of instantaneous capture 关Eq. 9 of Ref. 7兴. 63.8 kA/ cm2 is the optimum value of j0 maximizing −3 dB for the case of instantaneous capture and, max correspondingly, the top horizontal line shows −3 dB for that case 关Eq. 共11兲兴. T = 300 K and L = 1.1 mm. = 6.11⫻ 1010 cm−2, and an ideal overlap between the electron and hole wave functions in a QD. At these parameters, the maximum modal gain in a single-QD-layer structure gmax = 29.52 cm−1. The OCL thickness b = 0.28 m and the cavity length L = 1.1 mm 共at this L and the as-cleaved facet reflectivity R = 0.32, the mirror loss  = 10 cm−1兲. The modulation bandwidth depends strongly on the capture cross-section n. At a fixed j0, with making slower the capture into QDs 共reducing n兲, −3 dB decreases and finally becomes zero 共Figs. 2 and 3兲. As seen from Fig. 3, −3 dB = 0 at a certain nonvanishing value min n . This is due to the fact that, at a given j 0, no lasing is attainable in the structure if n ⬍ min n . Indeed, while j 0 is fixed, the threshold current density increases with decreasing n 共the curve corresponding to the left axis兲, jth = 冉 2 f n0 1 f n0 eNS 2 f n0 + ebB n1 + QD 1 − f n0 nvnQD 1 − f n0 冊 2 , 共7兲 where f n,0 is given by Eq. 共5兲. In order for the lasing to occur, j0 should be higher than jth. At a certain min n , j th becomes equal to j0 共Fig. 3兲. At n ⱕ min , j ⱖ j , th 0 which n means that there can be no lasing and hence no direct modulation in the structure 共the shaded region in Fig. 3兲. The minimum tolerable n for the lasing to occur at j0 is found from the condition jth = j0 and is given by 冑 j0 − eNS 2 f + QD n0 冑 eq jth − eNS 2 f QD n0 As seen from Eq. 共5兲, the confined-carrier level1 冑ebB min , n 共j 0兲 = eq occupancy f n,0 in a QD at the steady-state is pinned at its vnQD 1 − f n0 j0 − jth threshold value and does not change with j0 above the lasing 共8兲 threshold. In contrast to f n,0, the steady-state free-carrier deneq eq where jth is jth for the case of instantaneous capture 关jth is sity nOCL,0 in the OCL is not pinned—it rises with j0 above obtained using n = ⬁ in Eq. 共7兲兴. the lasing threshold. It should be emphasized that it is the noninstantaneous capture of carriers from the OCL into QDs that causes this rise in nOCL,0 above the lasing threshold.10,11 We obtain from Eqs. 共1兲–共3兲 a set of algebraic equations in the frequency-dependent small amplitudes ␦nOCL−m, ␦ f n−m, and ␦nph−m, the solution of which yields the modulation response function H共兲 = 兩␦nph−m共兲 / ␦nph−m共0兲兩2. Finally, we arrive at a cubic equation for the square of the modulation bandwidth −3 dB—the frequency, at which H共兲 has fallen to half its dc 共 = 0兲 value. For an illustration of our results, room-temperature operation of a GaInAsP heterostructure lasing near 1.55 m 共Ref. 8兲 is considered here. We assume 10% QD-size flucFIG. 3. Modulation bandwidth 共at a very low j0兲 and threshold current tuations, the surface density of article. QDs in a single-layer density vs terms captureat:cross-section into a QD in a single-layer structure. This article is copyrighted as indicated in the Reuse of AIP contentNisS subject to the http://scitation.aip.org/termsconditions. Downloaded to IP: f 2n0 128.173.125.76 On: Tue, 01 Apr 2014 19:24:05 131108-3 Appl. Phys. Lett. 98, 131108 共2011兲 Asryan, Wu, and Suris (GHz) 20 ω-3 dB / 2π 2 10 共−3 j0 (kA/cm ) (5 QD-layers) 10 0 20 ⬀ where −3 5 QD-layers Single QD-layer 50 100 j0 (kA/cm ) (Single QD-layer) 2 FIG. 4. Modulation bandwidth vs dc component of the injection current density in single- and 5-QD-layer-structures. A plausible value n = 10−11 cm2 共Refs. 14 and 15兲 of the capture cross-section is used. As seen from Eq. 共8兲, when j0 decreases and approaches min , increases infinitely, i.e., no lasing is attainable at jeq th n eq j0 ⱕ jth even if the carrier capture into QDs is instantaneous. With increasing j0, min n becomes smaller, i.e., the lasing can occur and hence the direct modulation of the output power is possible at a slower capture. At high j0 共when min n → 0兲, the asymptotic expression for −3 dB for n in the min 关共n − min vicinity of min n n 兲 / n Ⰶ 1兴 is dB ⬇ 2冑r − 1vggmax f n0共1 − f n0兲 n − min n , 2 − f n0 min n 共9兲 / 2π ω -3max dB (GHz) where the numerical parameter r = 100.3 ⬇ 1.995 originates from the definition of the ⫺3 dB bandwidth, 10 log10 H共−3 dB兲 = −3. As a function of the dc component j0 of the injection current density, −3 dB has a maximum 共Fig. 4兲. In a singleQD-layer structure 共the dotted curve兲, the optimum value jopt max max of j0, at which −3 dB is attained, is very high, i.e., −3 dB is unattainable. As seen from the figure, there are the following two advantages in a multi-QD-layer structure 共the solid curve兲 as compared to a single-layer structure: 共i兲 −3 dB is considerably higher at the same j0 and 共ii兲 jopt is considerably max reduced, which means that −3 dB is practically attainable. At large n, when capt,0 / ph Ⰶ 1 关capt,0 and ph are given by Eqs. 共4兲 and 共6兲, respectively兴, both −3 dB at a given j0 max 共Fig. 2兲 and −3 dB 共Fig. 5兲 asymptotically approach their saturation values 共the horizontal dashed lines兲 corresponding to the case of instantaneous capture into QDs, 20 5 QD-layers Single QD-layer 10 0 -14 10 10 -12 σ n (cm 10 2 − −3 -10 ) FIG. 5. Maximum modulation bandwidth vs capture cross-section into a max QD. The horizontal dashed line shows −3 dB for the case of instantaneous capture into QDs 关Eq. 共11兲兴. dB兲, max max 共−3 dB兩n=⬁ − −3 dB兲 capt,0 1 ⬀ , ph n dB 兩n=⬁ max −3 dB兩n=⬁ ⬇ 0 0 −3 dB兩n=⬁ 共10兲 is given by Eq. 9 of Ref. 7 and 冑2 ph . 共11兲 max As seen from Fig. 5, while the saturation value of −3 dB at n → ⬁ and at a fixed L 关Eq. 共11兲兴 does not depend on the max number of QD-layers, −3 dB at a given finite n is higher in a multilayer structure as compared to a single-layer structure. In conclusion, we have shown that the carrier capture from the OCL into QDs can strongly limit the modulation bandwidth −3 dB of a QD laser. −3 dB is highest in the case of instantaneous capture into QDs, when the cross-section of carrier capture into a QD n = ⬁. With reducing n, −3 dB decreases and becomes zero at a certain nonvanishing min n . This min n presents the minimum tolerable n for the lasing to occur at a given dc component j0 of the injection current density. The use of multiple-layers with QDs has been shown to significantly improve the modulation response of the laser—−3 dB is considerably higher in a multilayer structure as compared to a single-layer structure at the same j0. At a plausible cross-section n = 10−11 cm2,14,15 −3 dB as high as 19 GHz can be obtained in a 5-QD-layer structure with the cavity length L = 1.1 mm at a practical value of j0 = 7 kA/ cm2. Our analysis provides a basis for optimizing the QD laser design for high-speed operation. L.V.A. and Y.W. acknowledge the U.S. Army Research Office 共Grant No. W911-NF-08-1-0462兲, Y.W. also acknowledges the China Scholarship Council, and R.A.S. acknowledges the Russian Foundation for Basic Research 共Grant No. 08-02-01337兲 and the Program “Fundamental Research in Nanotechnology and Nanomaterials” of the Presidium of the Russian Academy of Sciences for support of this work. R. Dingle and C. H. Henry, U.S. Patent No. 3982207 共21 September 1976兲. 2 Zh. I. Alferov, Rev. Mod. Phys. 73, 767 共2001兲. 3 W. T. Tsang, Appl. Phys. Lett. 40, 217 共1982兲. 4 P. S. Zory, Jr., Quantum Well Lasers 共Academic, Boston, 1993兲. 5 Y. Arakawa and H. Sakaki, Appl. Phys. Lett. 40, 939 共1982兲. 6 A. E. Zhukov, A. R. Kovsh, S. S. Mikhrin, A. P. Vasil’ev, E. S. Semenova, N. A. Maleev, V. M. Ustinov, M. M. Kulagina, E. V. Nikitina, I. P. Soshnikov, Y. M. Shernyakov, D. A. Livshits, N. V. Kryjanovskaya, D. S. Sizov, M. V. Maximov, A. F. Tsatsul’nikov, N. N. Ledentsov, D. Bimberg, and Zh. I. 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