Graz Advanced School of Science PHYSICS COLLOQUIUM OF THE UNIVERSITY OF GRAZ AND THE GRAZ UNIVERSITY OF TECHNOLOGY Dr. Ralph Ernstorfer Max Planck Research Group for Structural & Electronic Surface Dynamics Fritz-Haber-Institut der Max-Planck-Gesellschaft, Berlin, Germany http://w0.rz-berlin.mpg.de/pc/ernstorfer Electronic and Structural Dynamics in Solids: A Momentum-Resolved View on Microscopic Coupling and Correlation Phenomena Abstract: The coupling and mutual dependence of electronic and vibrational degrees of freedom is at the heart of microscopic as well as macroscopic phenomena in condensed matter. Ultrafast pump-probe techniques provide experimental access to these coupling and correlation effects by revealing the microscopic response to specific excitation of a material. In particular, we employ time- and angle-resolved photoelectron spectroscopy (trARPES) and femtosecond electron diffraction (FED) [1] and imaging [2] in order to obtain a momentum-resolved view on the dynamics of electrons and phonons. I will discuss electron-lattice interaction and electron dynamics in two classes of materials. First, the electron-phonon coupling in the free-electron metal aluminium is revisited and quantitatively investigated with FED and first-principle calculations. Our results challenge the validity of the twotemperature approximation and we propose a refined non-thermal lattice model [3]. Second, I will discuss ultrafast electron and phonon dynamics in the semiconducting transition metal dichalcogenide WSe2. TrARPES with fs XUV pulses reveals the evolution of spin- and pseudospin-polarized excited states and allows for mapping of the conduction band structure in the entire Brillouin zone. The complementary momentum-resolved dynamics of phonons in this material is studied by FED. [1] [2] [3] [4] L. Waldecker et al., J. Appl. Phys. 117, 044903 (2015). M. Müller et al., Nature Communications 5, 5292 (2014). M. Müller et al., ACS Photonics 3, 611 (2016). L. Waldecker et al., Phys. Rev. X 6, 021003 (2016). R. Bertoni et al., arXiv:1606.03218. Termin: Ort: Dienstag, 21.6.2016, 17.00 Uhr KFU Graz KFU Graz, Universitätsplatz 5, Hörsaal 05.01, Meet-the-speaker ab 16.30 Uhr, Bibliothek des FB Experimentalphysik, 1. Stock, ZiNr.: 122 Gastgeber: Univ.-Prof. Dr. Martin Sterrer – Inst. f. Physik – Surface Science For a regularly updated colloquium program see: http://www.if.tugraz.at/colloquium.html
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