Lensless imaging based on coherent backscattering in random media Lei Xu, Hao Yang, Peilong Hong, Fang Bo, Jingjun Xu, and Guoquan Zhang Citation: AIP Advances 4, 087124 (2014); doi: 10.1063/1.4893471 View online: http://dx.doi.org/10.1063/1.4893471 View Table of Contents: http://scitation.aip.org/content/aip/journal/adva/4/8?ver=pdfcov Published by the AIP Publishing Articles you may be interested in Ultrabroadband generation of multiple concurrent nonlinear coherent interactions in random quadratic media Appl. Phys. Lett. 103, 101101 (2013); 10.1063/1.4819855 Optimizing photon sieves to approach Fresnel diffraction limit via pixel-based inverse lithography J. Vac. Sci. Technol. B 29, 041002 (2011); 10.1116/1.3605473 Observation of speckle patterns in extreme ultraviolet imaging J. Vac. Sci. Technol. B 19, 2406 (2001); 10.1116/1.1421550 Application of an inverse scattering technique to diffusive photon density images J. Appl. Phys. 88, 11 (2000); 10.1063/1.373617 Fluorescence microscopic imaging through tissue-like turbid media J. Appl. Phys. 87, 3214 (2000); 10.1063/1.372326 All article content, except where otherwise noted, is licensed under a Creative Commons Attribution 3.0 Unported license. See: http://creativecommons.org/licenses/by/3.0/ Downloaded to IP: 202.113.19.219 On: Sat, 16 Aug 2014 01:10:23 AIP ADVANCES 4, 087124 (2014) Lensless imaging based on coherent backscattering in random media Lei Xu, Hao Yang, Peilong Hong, Fang Bo, Jingjun Xu, and Guoquan Zhanga The MOE Key Laboratory of Weak Light Nonlinear Photonics, School of Physics and TEDA Applied Physics Institute, Nankai University, Tianjin 300457, China (Received 10 May 2014; accepted 7 August 2014; published online 15 August 2014) We studied lensless imaging due to coherent backscattering in random media both theoretically and experimentally. The point spread function of the lensless imaging system was derived. Parameters such as the volume fraction of the scatterer in the random scattering medium, the diameter of the scatterer, the distance between the object to be imaged and the surface of the random scattering medium were optimized to improve the image contrast and resolution. Moreover, for complicated objects, high contrast and quality images were achieved through the high-order intensity correlation measurement on the image plane, which may propel this imaging technique C 2014 Author(s). All article content, except where otherto practical applications. wise noted, is licensed under a Creative Commons Attribution 3.0 Unported License. [http://dx.doi.org/10.1063/1.4893471] I. INTRODUCTION The phenomena and effects of light propagation in disordered media, such as coherent backscattering1–3 and Anderson localization,4, 5 have been studied intensively.6–10 In recent years, random scattering, which is always thought as noise and fundamental limit for an optical system in the past,11–13 has been used for image formation.14–16 Furthermore, researchers found the random scattering useful to overcome the diffraction limit and perform wide-area imaging.17, 18 By calculating the transmission matrix, Gigan et al. have achieved a rapid and accurate reconstruction of an arbitrary image after transmitting through a complex medium.19 Lensless imaging has been demonstrated based on the coherent backscattering from random scattering media without the requirement to know the inner properties of multiple scattering of light within such random media.14, 15 However, for complicated objects, low image contrast makes this imaging technique almost impossible to be put into practice (the image contrast is defined as γ = Iim /Ibg , where Iim and Ibg are the intensities related to the image and background in the image plane, respectively). Therefore, efficient and effective methods to improve the image contrast are urgently needed in practice. In this paper, we carried out a detailed study on this lensless imaging due to coherent backscattering in random media. The point spread function (PSF) of the lensless imaging system was derived theoretically. The image resolution and contrast were optimized by adjusting the parameters of the random media and the imaging system. Finally, we demonstrated that the image quality can be improved significantly by measuring the high-order intensity correlation function in the image plane. II. THEORETICAL ANALYSIS When a light source illuminates a random scattering medium, the light waves scattered multiply by the medium will form the image of the light source at the equivalent backward source position a Electronic mail: [email protected] 2158-3226/2014/4(8)/087124/11 4, 087124-1 C Author(s) 2014 All article content, except where otherwise noted, is licensed under a Creative Commons Attribution 3.0 Unported license. See: http://creativecommons.org/licenses/by/3.0/ Downloaded to IP: 202.113.19.219 On: Sat, 16 Aug 2014 01:10:23 087124-2 Xu et al. AIP Advances 4, 087124 (2014) FIG. 1. Geometry used for the calculation of PSF, showing two interfering light paths p1 and p2 . S is the point source. The light is incident on the random scattering medium, and the backscattered light Si at different position is recorded. due to coherent backscattering, as depicted in Fig. 1. In the simplest case with a point source S, the fundamental features of the lensless imaging system are characterized by the PSF, which is the intensity distribution in the image plane formed by the coherent backscattering from the semiinfinite random scattering medium. Therefore, the instantaneous PSF can be defined as the ratio of the time-dependent emergent energy in the image plane to the incident energy flux of the point source. According to Refs. 7 and 11, let’s first consider the dynamic case in which an energy pulse from the point source impinges on a random scattering medium with random motion particles, the associated PSF of the lensless imaging based on coherent backscattering from a semi-infinite random scattering medium can be written as c r1 , rn ; t) dz 1 dz n d 2r1 d 2 ρ P( PSF(s , si ; t) = 2 2 l d r1 z 1 − μ(sz,1r )l − μ(szn,r )l − 1 − zn i n 1 e + e μ(si ,r1 )l μ(s ,rn )l × 2 z z 1 −1 + zn + 1 + zn +e 2 μ(s ,r1 )l μ(si ,rn )l μ(si ,r1 )l μ(s,rn )l cos (s , si ; r1 , rn ) , (1) where P( r1 , rn ; t) is the Green’s function which describes the light transport from a pulse located at r1 at time t0 = 0 to rn at time t. For a large number of random scatterers, it is well approximated by the solution of a time-dependent diffusion equation,6, 7 and can be expressed approximately in the 2 −(z−z )2 /4D t 2 e−ρ /4Dd t n d e −e−(z+zn +2z0 ) /4Dd t . l is the elastic mean free path of the form P( r1 , rn ; t) = (4π Dd t)3/2 random scattering medium, c is the light speed in vacuum, z0 = 2/3l, Dd is the diffusion constant, r1 and rn are the positions of the first and the last nth scatterers in the random scattering medium, ρ = ( r1 − rn )⊥ is the projection of r1 − rn on the interface plane, d 2 r1 and d 2 ρ depict the energy integration over the incident and emergent surfaces, respectively. μ(si , r1,n ) are the projections of → − → − → −→ −→ −→ −→ − →/|− sr 1 sr 1 |, sr n /|sr n |, si r 1 /|si r 1 |, si r n /|si r n | on the z-axis, respectively. d is the distance between the point source and the surface of the random scattering medium, r is the displacement of si from s, (s , si ; r1 , rn ) is the net phase difference between two counterpropagating paths p1 and p2 , as shown r1 ) and in Fig. 1. In the case when r d, one can take the approximation μ(s , r1 ) = μ(si , r1 ) = μ( All article content, except where otherwise noted, is licensed under a Creative Commons Attribution 3.0 Unported license. See: http://creativecommons.org/licenses/by/3.0/ Downloaded to IP: 202.113.19.219 On: Sat, 16 Aug 2014 01:10:23 087124-3 Xu et al. AIP Advances 4, 087124 (2014) μ(s , rn ) = μ(si , rn ) = μ( rn ). Thus, Eq. (1) is reduced as c PSF(s , si ; t) = 2 r1 , rn ; t) dz 1 dz n d 2r1 d 2 ρ P( l d 2r1 z − 1 − zn ×e μ(r1 )l μ(rn )l 1 + cos (s , si ; r1 , rn ) . (2) According to Refs. 6, 7, and 11, the stationary PSF can be obtained by integrating Eq. (2) over time, which, in fact, can be done by integrating P( r1 , rn ; t) over time, and one gets P( r1 , rn , ρ) = P( r1 , rn ; t)dt 1 = 4π Dd 1 1 − |ρ| 2 + (z − z n )2 |ρ| 2 + (z + z n + 2z 0 )2 So the stationary PSF can be written as PSF(s , si ) = l2 ×e c d 2r1 . (3) z r1 , rn , ρ) dz 1 dz n d 2r1 d 2 ρ P( − μ(r1 )l − μ(zrnn )l 1 1 + cos (s , si ; r1 , rn ) , (4) where μ( r1 ) = cos θ1 and μ( rn ) = cos θn . Such a stationary PSF can be experimentally evaluated with a continuous wave incident light, just as the cases in Refs. 6 and 7. The expression of stationary PSF can be further simplified when one considers the condition in Ref. 6, where r1 and rn are located on the same plane at z = l. In this case, the PSF can be simplified as 1 1 − 1 2 2 − PSF(s , si ) = A d r1 d ρ e cos θ1 2 2 |ρ| |ρ| +a 1 ×e− cos θn 1 + cos (s , si ; r1 , rn ) , (5) →+− where A is a constant, a = 2(l + z0 ), and the net phase difference (s , si ; r1 , rn ) = 2π [(− sr si→ rn ) − 1 λ − → − → (srn + si r1 )]. Considering the on-axis condition (when r is far away from the axis, P → 0), and r d, the net phase difference can be written as 2π rs − rsi ) ( r1 − rn ) · ( λd 2π ρ · r , = λd (s , si ; r1 , rn ) = (6) and d cos θn = , d 2 + (d tan θ1 )2 + |ρ| 2 − 2d|ρ| tan θ1 cos φ →. Therefore, the stationary PSF can be written as where φ is the angle between ρ and − ss i 1 1 − 1 2 2 − PSF(s , si ) = A d r1 d ρ e cos θ1 |ρ| |ρ| 2 + a2 2π − cos1θn 1 + cos ×e ρ · r . λd (7) (8) According to Eq. (8), a theoretical image profile of a point source at the equivalent backward source position is shown in Fig. 2, showing the one-to-one correspondence between the point source and its image. Suppose that there is an arbitrary object with a transmission profile T (s ), the intensity distribution in the image plane will be proportional to T (s )ds + (PSFnorm − 1)T (s ), All article content, except where otherwise noted, is licensed under a Creative Commons Attribution 3.0 Unported license. See: http://creativecommons.org/licenses/by/3.0/ Downloaded to IP: 202.113.19.219 On: Sat, 16 Aug 2014 01:10:23 087124-4 Xu et al. AIP Advances 4, 087124 (2014) FIG. 2. The theoretical image profile PSF (normalized to the background) of a point source calculated according to Eq. (8). The wavelength of the incident light is set to be 532 nm, d = 23 cm, and l = 35.4 μm, respectively. where T (s )ds represents the total background on the image plane and PSFnorm is the PSF of a single point source normalized to its background as shown in Fig. 2. It is evident that the image contrast will be extremely low and the image may even be indiscernible for a complicated object, which should be overcome in practical application. III. EXPERIMENTAL RESULTS AND DISCUSSIONS In this section, we will give an experimental demonstration of the above theoretical analysis about this lensless imaging technique. Then we will optimize the material parameters of the random medium to optimize the image quality and contrast. Finally, we demonstrate a significant improvement on the image contrast by performing the high-order intensity correlation measurement at the image plane. A. Experimental scheme Figure 3 shows the schematic diagram of the lensless image system based on the coherent backscattering in a random medium. A 532-nm laser beam was focused by a lens with a focal length of 6 cm onto a 10-μm pinhole template to mimic a 10-μm-diameter point source. The total power of the light emerging from the object was set to be 100 mW in the following. Then the diverging light passed through a 50:50 beam splitter and impinged on a random scattering medium, which was the suspension of polystyrene spheres dispersed in deionized water in our experiments. The backward scatterings from the random scattering medium were reflected by the beam splitter. A charge coupled device (CCD) camera was placed at the equivalent backward source position to record the intensity distribution of the backscattered light there. The exposure time of CCD was set to be 0.04 ms for each image frame, which is much less than the characteristic time of 1 ms associated with the Brownian motion of the scatters (polystyrene spheres).7 Considering the de-polarization effect of the multiple scattering of light,1, 2, 6 a polarization analyzer (P) was placed just before the CCD camera so that All article content, except where otherwise noted, is licensed under a Creative Commons Attribution 3.0 Unported license. See: http://creativecommons.org/licenses/by/3.0/ Downloaded to IP: 202.113.19.219 On: Sat, 16 Aug 2014 01:10:23 087124-5 Xu et al. AIP Advances 4, 087124 (2014) FIG. 3. Experimental configuration for the observation of lensless imaging due to coherent backscattering in a random medium. Here S stands for the object to be imaged, Si is the image, BS is beam splitter, P is the polarization analyzer, respectively. only the light scattering with its polarization parallel to that of the incident light was allowed to pass through. In this way, one can get a higher image contrast. This is because the enhancement factor is larger for the scattered light polarized parallel to the incident light than that polarized vertically to the incident light, which may be due to the angular dependence of the light scattered from each individual scatterer in the random scattering medium.1, 2, 6 The distance d between the object (point source) and the surface of the random scattering medium was set to be 23 cm unless stated elsewhere. In order to suppress the fluctuations due to random interference of light among multiply scattered paths, the image profile, under the condition of ergodicity,7, 20 could be ensemble-averaged over 100,000 frames in the following.1–3 B. Characterization and optimization A typical image of a point-source object, obtained through suspension of polystyrene spheres with a 1.0-μm diameter and a volume fraction ϕ being 5 vol.%, is shown in Fig. 4(a). The thickness of the random medium sample was 16 mm. The red curve in Fig. 4(b) is a theoretical fit to the measured experimental data (the solid squares) according to Eq. (8). The elastic mean free path l was measured to be 35.4 μm by the coherent backscattering experiment.21 Quantitative agreement is achieved between the theoretical prediction and the experimental data, with the exception that the measured enhancement factor is less than 2. This is due to several factors such as a non-ideal point source, a finite sample cell size (which eliminates the possibility of long scattering paths), and the presence of closed loop scattering paths.20, 21 The resolution and quality of the image depends on several factors, such as the volume fraction of the scatterer ϕ, the diameter of the scatterer D, and the distance d. When the scatterer diameter D is fixed, low volume fraction ϕ (corresponding to a low number content) reduces the possibility of multiple scattering paths, and therefore resulting in a small enhancement factor. On the other hand, when the volume fraction is too large (corresponding to a large number content), the recurrent scattering leads to a reduction of the enhancement factor and an increase in the full width at halfmaximum (FWHM) of the PSF,22 which lead to a decreasing image resolution. The scattering strength increases with increasing diameter D in general, meanwhile, the number content decreases for a fixed volume fraction ϕ, thus reducing the possible paths of the multiple scattering of light which forms the image at the equivalent backward source position. Therefore, one has to optimize the scatterer diameter D to balance these two effects to improve the image contrast. Also, the FWHM increases with increasing volume fraction of polystyrene spheres, which will result in a reduction in All article content, except where otherwise noted, is licensed under a Creative Commons Attribution 3.0 Unported license. See: http://creativecommons.org/licenses/by/3.0/ Downloaded to IP: 202.113.19.219 On: Sat, 16 Aug 2014 01:10:23 087124-6 Xu et al. AIP Advances 4, 087124 (2014) (a) (b) FIG. 4. The image of a one-point source at the equivalent backward source position. (a) is the 2-dimensional image and (b) is the image profile across the image center. The solid squares in (b) are the measured data, while the red solid curve is a theoretical fit to the experimental data according to Eq. (8). FIG. 5. The normalized image profiles of a point-source object for suspensions of 1.0 μm-diameter polystyrene spheres with ϕ being 2 vol.% (dark solid curve), 5 vol.% (red dashed curve), and 8 vol.% (blue dotted curve), respectively. the image resolution. The corresponding experimental results are shown in Figs. 5 and 6. Here, Fig. 5 gives the image profiles of a point source with three different volume fraction of polystyrene spheres of 1.0 μm-diameter, and Fig. 6 gives the dependence of the enhancement factor on the scatterer’s diameter D with various volume fraction ϕ, respectively. One sees that the image contrast is relatively high when the diameter of spheres ranging from 0.5 μm to 1.2 μm in general. Referring to these results, in order to get better image resolution and quality, we chose a suspension of polystyrene spheres with a sphere diameter of 1.0 μm and a volume fraction of 5 vol.% as the random scattering medium in the following experiments. One should note that the above optimized conditions are valid only for the suspension of polystyrene spheres used in our experiments because different scatterers All article content, except where otherwise noted, is licensed under a Creative Commons Attribution 3.0 Unported license. See: http://creativecommons.org/licenses/by/3.0/ Downloaded to IP: 202.113.19.219 On: Sat, 16 Aug 2014 01:10:23 087124-7 Xu et al. AIP Advances 4, 087124 (2014) FIG. 6. The dependence of the enhancement factor on the scatterer diameter D for suspensions of polystyrene spheres with ϕ being 2 vol.% (black solid squares), 5 vol.% (red solid circles), and 8 vol.% (blue solid triangles), respectively. The lines are guided by eyes. or particles will have different scattering properties, nevertheless, the optimization procedure to get the best performance is similar. Figure 7 shows the image profiles of PSF at different distances d, which are not sensitive to the distance d. This indicates that one can get images with unit magnification within a large range of distance d. The slight decrease in the enhancement factor for large d may be due to the fact that less light (emerging from the point source) is injected into the random scattering medium to participate in the coherent backscattering effect with increasing d because of the finite sample size in the experiment. C. Image contrast improved by the high-order intensity correlation As we have mentioned above, the image contrast for a complicated object will be extremely low and even indiscernible because of the relatively high background, this puts a serious limitation on this novel technique for practical applications. Here we employed the high-order intensity correlation measurement on the equivalent backward source plane to improve the image contrast. Our results show that this lensless imaging based on coherent backscattering with high-order intensity correlation method is linear and the image contrast can be significantly improved for a complicated object, which may propel this novel technique for potential image applications. The Nth-order spatial intensity correlation function is defined as23–25 G (N ) (r1 , . . . , r N ) = I1 (r1 ) . . . I N (r N ) , (9) where Ij (rj ) gives the intensity at position rj , and . . . stands for an ensemble average. In our case, we consider the intensity correlation function under the condition r1 = r2 = . . . = rj = r, which is also called as the Nth-order moment of intensity, and it can be written as G (N ) (r ) = I (r ) N . (10) All article content, except where otherwise noted, is licensed under a Creative Commons Attribution 3.0 Unported license. See: http://creativecommons.org/licenses/by/3.0/ Downloaded to IP: 202.113.19.219 On: Sat, 16 Aug 2014 01:10:23 087124-8 Xu et al. AIP Advances 4, 087124 (2014) FIG. 7. The normalized image profiles of a point-source object with distance d being 23 cm (black solid curve), 33 cm (red dotted curve), 43 cm (blue dash-dotted curve), and 53 cm (pink dashed curve), respectively. A suspension of polystyrene spheres with a sphere diameter of 1.0 μm and a volume fraction of 5 vol.% was used in the experiment. As alreadyshown in Sec. II, the image of an arbitrary object with a transmission profile T (s ) is proportional to T (s )ds + (PSFnorm − 1)T (s ), where the first term T (s )ds corresponds to the total background Ibg and the second term (PSFnorm − 1)T (s ) depicts the useful net image information Iim − Ibg on the image plane. Here Iim depicts the averaged intensity distribution at the image position, and Ibg is the averaged background intensity far away from the image position in the image plane. The image contrast becomes γN = = (N ) G im ) G (N bg N Iim N Ibg = 1+ N N − Ibg Iim N Ibg . (11) For complicated objects, the image will be submerged in the background noise in the image plane, and the intensity difference between the image and the background is very small and both the image and background beams experience the same statistically random scattering process so that the corresponding normalized Nth-order intensity correlation functions in the image plane are the same, namely N N Ibg Iim = = g, N Iim Ibg N (12) All article content, except where otherwise noted, is licensed under a Creative Commons Attribution 3.0 Unported license. See: http://creativecommons.org/licenses/by/3.0/ Downloaded to IP: 202.113.19.219 On: Sat, 16 Aug 2014 01:10:23 087124-9 Xu et al. AIP Advances 4, 087124 (2014) FIG. 8. The normalized image profile of a three-point-source object (point1, point2, and point3 with an input intensity ratio of 8 : 2 : 1). which is also confirmed experimentally. By substituting Eq. (12) into Eq. (11), γ N can be further written as γN = 1 + = = ≈ = N N − Ibg Iim N Ibg g Iim N − Ibg N 1+ gIbg N Iim − Ibg N 1 N N 1+ − Ibg Ibg 1 + Ibg N Ibg Iim − Ibg 1 N N Ibg 1 + N − Ibg 1+ Ibg N Ibg Iim − Ibg . 1+ N Ibg (13) It is seen from Eq. (13) that, by performing the Nth-order intensity correlation measurement, one expects to amplify the intensity difference between the image and the background by N times. Therefore, the image contrast γ N can be improved dramatically. Eq. (13) also shows that the net image strength Iim − Ibg increases linearly with the increase of the correlation order N, which clearly indicates that the imaging system is linear. One should also note that the imaging system is nonlinear when the net image term is comparable to the background term. All article content, except where otherwise noted, is licensed under a Creative Commons Attribution 3.0 Unported license. See: http://creativecommons.org/licenses/by/3.0/ Downloaded to IP: 202.113.19.219 On: Sat, 16 Aug 2014 01:10:23 087124-10 Xu et al. AIP Advances 4, 087124 (2014) (a) (b) FIG. 9. (a) The 4th-order intensity correlation function of the image shown in Fig. 8, and (b) the net image strength of three points as a function of the correlation order N. Note that the net image strength of point2 and point3 are multipled by a factor of 10 in (b). (a) (b) FIG. 10. Images of an object ‘2’. (a) is the normalized image profile, and (b) is the image formed by performing the 8th-order intensity correlation measurement on the image plane, respectively. In the following, we will measure the intensity correlation function G(N) for the images of two objects: a three-point-source object and a number ‘2’ object. Note that, although we employed a coherent laser to illuminate the object, the spatial coherence between different points of the object will be totally washed out on the image plane because of the multiple scattering in the random scattering media, which can be easily confirmed experimentally. Figure 8 shows the normalized image profiles of the three point sources (point1, point2 and point3) with an input intensity ratio of 8 : 2 : 1. The enhancement factors of these three point sources on the image plane were measured to be 1.48, 1.11 and 1.06, respectively. The ratio of net image strength among them is 8 : 1.8 : 1, which indicates that the imaging system based on coherent backscattering itself is linear. Figure 9(a) is the 4th-order intensity correlation function of the image shown in Fig. 8, and Fig. 9(b) is the net image strength of the Nth-order intensity correlation function as a function of the intensity correlation order N. It is clearly seen that the strength of the strongest one (point1), in which the strength of its image term in Fig. 8 is comparable to the background, increases nonlinearly with the increase of the correlation order N. More interestingly, the strengthes of the two weak ones (point2 and point3), in which the image term itself is much less than the background, increase linearly with All article content, except where otherwise noted, is licensed under a Creative Commons Attribution 3.0 Unported license. See: http://creativecommons.org/licenses/by/3.0/ Downloaded to IP: 202.113.19.219 On: Sat, 16 Aug 2014 01:10:23 087124-11 Xu et al. AIP Advances 4, 087124 (2014) the increase of the correlation order N, indicating that the imaging system with high-order intensity correlation method is linear as predicted theoretically. Note that the net image strengthes for the two weak points (point2 and point3) are multiplied by a factor of 10 in Fig. 9(b) for comparison. Figure 10(a) is the normalized image profile of a number ‘2’. It is seen that the image contrast is very low and it is difficult for one to identify the number ‘2’ in the image plane. Figure 10(b) is the result by measuring the 8th-order intensity correlation function on the image plane. One sees that the image contrast increases greatly and the image of the number ‘2’ is clearly displayed. This proves that the method is reliable for improving the quality of image based on coherent backscattering in a random medium. IV. CONCLUSIONS In summary, we have studied the lensless imaging based on the coherent backscattering effect of random scattering media, and gotten the PSF of this lensless imaging system. We have shown that the image contrast and resolution depend on several factors such as the diameter of the scatterer, the volume fraction of the suspension, the distance between the object and the surface of the random scattering medium. The contrast is relatively higher for suspension of polystyrene spheres with the sphere diameter between 0.5 μm to 1.2 μm dispersed in water. An increase in volume fraction of scatterers may increase the possible paths of multiple scattering of light, but meanwhile it increases the possibility of recurrent scattering, which may reduce the image contrast. Furthermore, we have demonstrated that the lensless imaging based on coherent backscattering with high-order intensity correlation method is linear for complicated objects, and the image quality can be significantly improved by performing the high-order intensity correlation measurement on the image plane. Therefore, this imaging technique could be practical even for complicated objects. ACKNOWLEDGMENTS This work is supported by the 973 program (2013CB328702), the NSFC (11174153 and 11374165), the 111 project (B07013), and the Fundamental Research Funds for the Central Universities. 1 P. E. Wolf and G. Maret, Phys. Rev. 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